Multiple scattering of light by atoms with internal degeneracy

An analytical microscopic theory for the resonant multiple scattering of light by cold atoms with arbitrary internal degeneracy is presented. It permits to calculate the average amplitude and the average intensity for one-photon states of the full transverse electromagnetic field in a dilute medium of unpolarized atoms. Special emphasis is laid upon an analysis in terms of irreducible representations of the rotation group. It allows to sum explicitly the ladder and maximally crossed diagrams, giving the average intensity in the Boltzmann approximation and the interference corrections responsible for weak localization and coherent backscattering. The exact decomposition into field modes shows that the atomic internal degeneracy contributes to the depolarization of the average intensity and suppresses the interference corrections. Static as well as dynamic quantities like the transport velocity, diffusion constants and relaxation times for all field modes and all atomic transitions are derived.Comment: Corrected minor errors. Slightly extended version of the article appeared in prin

Comment on ``Intensity correlations and mesoscopic fluctuations of diffusing photons in cold atoms''

In a recent Letter (Phys. Rev. Lett. \textbf{98}, 083601 (2007), arXiv:cond-mat/0610804), O. Assaf and E. Akkermans claim that the angular correlations of the light intensity scattered by a cloud of cold atoms with internal degeneracy (Zeeman sublevels) of the ground state overcome the usual Rayleigh law. More precisely, they found that they become exponentially large with the size of the sample. In what follows, we will explain why their results are wrong and, in contrary, why the internal degeneracy leads to lower intensity correlations.Comment: 1 page. Comment submitted to PR

Coherent Backscattering with Nonlinear Atomic Scatterers

We study coherent backscattering of a quasi-monochromatic laser by a dilute gas of cold two-level atoms. We consider the perturbative regime of weak intensities, where nonlinear effects arise from {\em inelastic} two-photon scattering processes. Here, coherent backscattering can be formed by interference between {\em three} different scattering amplitudes. Consequently, if elastically scattered photons are filtered out from the photodetection signal by means of suitable frequency-selective detection, we find the nonlinear backscattering enhancement factor to exceed the linear barrier two.Comment: 4 pages, 3 figure

Mesoscopic scattering of spin s particles

Quantum effects in weakly disordered systems are governed by the properties of the elementary interaction between propagating particles and impurities. Long range mesoscopic effects due to multiple scattering are derived by iterating the single scattering vertex, which has to be appropriately diagonalized. In the present contribution, we present a systematic and detailed diagonalisation of the diffuson and cooperon vertices responsible for weak localisation effects. We obtain general expressions for eigenvalues and projectors onto eigenmodes, for any spin and arbitrary elementary interaction with impurities. This description provides a common frame for a unified theory of mesoscopic spin physics for electrons, photons, and other quantum particles. We treat in detail the case of spin-flip scattering of electrons by freely orientable magnetic impurities and briefly review the case of photon scattering from degenerate dipole transitions in cold atomic gases.Comment: published version, with a new figure and new section

Entanglement detection from interference fringes in atom-photon systems

A measurement scheme of atomic qubits pinned at given positions is studied by analyzing the interference pattern obtained when they emit photons spontaneously. In the case of two qubits, a well-known relation is revisited, in which the interference visibility is equal to the concurrence of the state in the infinite spatial separation limit of the qubits. By taking into account the super-radiant and sub-radiant effects, it is shown that a state tomography is possible when the qubit spatial separation is comparable to the wavelength of the atomic transition. In the case of three qubits, the relations between various entanglement measures and the interference visibility are studied, where the visibility is defined from the two-qubit case. A qualitative correspondence among these entanglement relations is discussed. In particular, it is shown that the interference visibility is directly related to the maximal bipartite negativity.Comment: 12 pages, 2 figures, published versio

Coherent Backscattering of Light with Nonlinear Atomic Scatterers

We study coherent backscattering of a monochromatic laser by a dilute gas of cold two-level atoms in the weakly nonlinear regime. The nonlinear response of the atoms results in a modification of both the average field propagation (nonlinear refractive index) and the scattering events. Using a perturbative approach, the nonlinear effects arise from inelastic two-photon scattering processes. We present a detailed diagrammatic derivation of the elastic and inelastic components of the backscattering signal both for scalar and vectorial photons. Especially, we show that the coherent backscattering phenomenon originates in some cases from the interference between three different scattering amplitudes. This is in marked contrast with the linear regime where it is due to the interference between two different scattering amplitudes. In particular we show that, if elastically scattered photons are filtered out from the photo-detection signal, the nonlinear backscattering enhancement factor exceeds the linear barrier two, consistently with a three-amplitude interference effect.Comment: 18 pages, 13 figures, submitted to Phys. Rev.

Light transport in cold atoms and thermal decoherence

By using the coherent backscattering interference effect, we investigate experimentally and theoretically how coherent transport of light inside a cold atomic vapour is affected by the residual motion of atomic scatterers. As the temperature of the atomic cloud increases, the interference contrast dramatically decreases emphazising the role of motion-induced decoherence for resonant scatterers even in the sub-Doppler regime of temperature. We derive analytical expressions for the corresponding coherence time.Comment: 4 pages - submitted to Physical Review Letter

Coherent light transport in a cold Strontium cloud

We study light coherent transport in the weak localization regime using magneto-optically cooled strontium atoms. The coherent backscattering cone is measured in the four polarization channels using light resonant with a J=0 to J=1 transition of the Strontium atom. We find an enhancement factor close to 2 in the helicity preserving channel, in agreement with theoretical predictions. This observation confirms the effect of internal structure as the key mechanism for the contrast reduction observed with an Rubidium cold cloud (see: Labeyrie et al., PRL 83, 5266 (1999)). Experimental results are in good agreement with Monte-Carlo simulations taking into account geometry effects.Comment: 4 pages, 2 figure